Hmm, it would be easier to give recommendations if you posted what your favourites are. What are your fave titles, genres? I have currently over 300 watched titles on MAL from a fair variety of genres, so maybe I could help?
As for my personal favourites, in no particular order: Gintama, Fullmetal Alchemist Brotherhood, Akira, Ghost in The Shell, Bungou Stray Dogs, Cowboy Bebop, Dorohedoro, Ergo Proxy, Parasyte, Mononoke (the series, not the Ghibli movie, tho that one is cool, too), Monster, No.6, Sidonia no Kishi, and I can go on and on. I can also recommend some less known stuff if you'd like to discover some hidden pearls or something?
I'm not mentioning decent anime that was based on manga where I consider manga way better (like Tokyo Ghoul, Noragami, or Akatsuki no Yona).